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  • A Comprehensive Review on Bilayer Tablets for Controlled Release Systems: Development, Issues and Future Prospects

  • Department Of Pharmaceutical Quality Assurance, Rajaram Bapu College Of Pharmacy, Kasegaon, Maharashtra, India 415404.

Abstract

Bilayer tablet technology has emerged as an advanced oral drug delivery strategy for achieving controlled, sustained, and combination drug release within a single dosage unit. The system allows incorporation of two incompatible drugs, separation of release profiles, and improvement in therapeutic efficacy and patient compliance. This review presents a comprehensive overview of bilayer tablets with emphasis on formulation strategies, excipient selection, manufacturing techniques, drug release mechanisms, evaluation methods, and therapeutic applications. The paper also discusses challenges associated with interlayer adhesion, compression parameters, scale-up, and regulatory aspects. Furthermore, the role of Quality by Design (QbD), Process Analytical Technology (PAT), and emerging industrial trends in enhancing bilayer tablet performance is critically analyzed. The review highlights recent advances and prospects in the development of bilayer tablets as a versatile platform for controlled release and fixed-dose combination therapies.

Keywords

Bilayer tablets; controlled release; fixed-dose combination; QbD; PAT; drug delivery; sustained release; pharmaceutical manufacturing

Introduction

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Oral drug delivery remains the most preferred route of administration due to its convenience, patient compliance, and cost-effectiveness. However, conventional dosage forms often fail to provide optimal therapeutic outcomes due to fluctuations in drug plasma concentration, frequent dosing requirements, and incompatibility between multiple active pharmaceutical ingredients. Bilayer tablet technology has emerged as a promising approach to overcome these limitations by integrating two drug layers or release profiles into a single dosage unit [1]. Bilayer tablets are designed to deliver drugs either simultaneously or sequentially through immediate-release and sustained-release mechanisms. This technology is particularly useful for combination therapy, chronotherapeutic delivery, and management of chronic diseases where multidrug therapy is required [2], [3]. The development of bilayer tablets has gained significant attention due to their ability to enhance therapeutic efficacy, improve patient adherence, and reduce dosing frequency. Nevertheless, the formulation and manufacturing of bilayer tablets involve complex challenges such as layer separation, compression optimization, and drug compatibility issues [4]. Recent research has focused on improving formulation strategies, evaluating excipient interactions, and addressing manufacturing challenges associated with bilayer tablet production [5], [6]. Academic and industrial investigations have also highlighted the importance of equipment design, process control, and polymer selection in achieving desired drug release profiles [7], [8]. Numerous case studies and formulation reports have demonstrated the application of bilayer tablets in various therapeutic areas, including cardiovascular disorders, diabetes, and gastrointestinal diseases [9], [10]. Additionally, industrial and academic repositories have provided valuable insights into manufacturing processes and equipment considerations for bilayer tablet development [11], [12].

Fundamentals of Bilayer Tablet Technology

Bilayer tablets consist of two distinct layers compressed into a single unit, each designed to perform a specific function such as immediate drug release, sustained release, or separation of incompatible active pharmaceutical ingredients. The concept is based on modifying drug release kinetics while maintaining mechanical integrity of the tablet [13]. The primary objective of bilayer technology is to achieve differential release patterns that can optimize therapeutic outcomes and reduce adverse effects. This can be achieved through appropriate selection of polymers, excipients, and compression techniques [14]. Bilayer systems are broadly categorized into sustained-release/immediate-release combinations, floating bilayer systems, and combination drug therapies. Each system is designed to meet specific pharmacokinetic and therapeutic requirements [15]. Industrial development of bilayer tablets involves careful consideration of powder flow, compressibility, and adhesion between layers. The success of bilayer technology largely depends on optimization of formulation variables and manufacturing parameters [16]. Recent academic contributions and methodological studies have provided detailed insights into formulation approaches and process development strategies for bilayer tablets [17], [18].

 

 

 

Figure 1: Conceptual drug release profile of bilayer tablet showing immediate and sustained drug release

 

Advantages and Disadvantages of Bilayer Tablets

Bilayer tablet technology offers several therapeutic and formulation advantages; however, certain technical and manufacturing limitations are also associated with this system. The major advantages and disadvantages reported in the literature are discussed below.

Advantages of Bilayer Tablets

  1. Combination therapy: Bilayer tablets allow incorporation of two active pharmaceutical ingredients within a single dosage form, which is particularly useful in the treatment of chronic diseases requiring multidrug therapy. [1,3]
  2. Separation of incompatible drugs: The bilayer system enables physical separation of drugs that may be chemically or physically incompatible, thereby improving formulation stability. [1,5]
  3. Dual drug release profiles: Bilayer tablets can provide immediate release from one layer and sustained or controlled release from the second layer, ensuring rapid onset followed by prolonged therapeutic action. [2,32]
  4. Improved patient compliance: By combining multiple drugs or release mechanisms in a single tablet, bilayer tablets reduce dosing frequency and improve patient adherence to treatment. [54,55]
  5. Enhanced therapeutic effectiveness: Controlled drug release helps maintain optimal plasma drug concentration for extended periods, minimizing fluctuations in drug levels. [31,33]
  6. Flexibility in formulation design: Different polymers, excipients, and release mechanisms can be incorporated into individual layers, allowing greater flexibility in drug delivery design. [19,20]
  7. Application in controlled and fixed-dose combination therapies: Bilayer tablets are widely used in the management of cardiovascular diseases, diabetes, and gastrointestinal disorders due to their ability to deliver multiple drugs effectively. [41,42]

Disadvantages of Bilayer Tablets

  1. Complex manufacturing process: Production of bilayer tablets requires specialized compression equipment and careful control of process parameters. [4,29]
  2. Scale-up challenges: Maintaining uniform layer weight, compression force, and powder flow during large-scale production can be difficult. [29]
  3. Risk of layer cross-contamination: Improper die filling or powder flow may cause mixing of layers, affecting drug release characteristics and dosage accuracy. [26,28]
  4. Moisture sensitivity: Environmental factors such as humidity may affect compressibility, interlayer bonding, and drug stability. [27,48]

Formulation Strategies and Excipients

Formulation design plays a critical role in determining the performance of bilayer tablets. Selection of suitable excipients ensures mechanical strength, drug stability, and controlled drug release. Polymers, binders, diluents, and disintegrants are carefully chosen to achieve desired functional properties [19]. Common polymers used include hydrophilic matrix formers such as HPMC, carbopol, and polyethylene oxide, which regulate drug release through swelling and diffusion mechanisms. Hydrophobic polymers may also be incorporated to modify release kinetics [20]. Floating bilayer tablets and gastro-retentive systems require specific excipients such as gas-generating agents and low-density polymers to maintain buoyancy and prolong gastric residence time [21]. Academic and industrial studies emphasize the importance of excipient compatibility and optimization of polymer ratios to ensure stability and performance of bilayer systems [22].

Regional journal publications and formulation studies have demonstrated diverse excipient combinations tailored to therapeutic requirements and manufacturing feasibility [23], [24].

 

 

 

Figure 2: Structure of bilayer tablet showing immediate and sustained release layers

 

Manufacturing Techniques & Equipment

Manufacturing of bilayer tablets requires specialized compression techniques capable of producing two distinct layers with adequate bonding. The process typically involves sequential filling and compression within a single die cavity [25]. Industrial equipment such as rotary bilayer tablet presses enables precise control of weight, compression force, and layer thickness. Advances in feeder design and automation have significantly improved manufacturing reproducibility [26]. Granulation techniques including wet granulation, dry granulation, and direct compression are commonly employed depending on drug and excipient properties [27].  Process optimization focuses on parameters such as compression force, dwell time, and powder flow to prevent delamination and ensure mechanical integrity [28]. Industrial reviews have highlighted scale-up challenges and process optimization strategies for large-scale bilayer tablet production [29].

Equipment innovations and automation technologies continue to enhance manufacturing efficiency and quality control [30]. In addition, pre-compression of the first layer is a critical step to provide sufficient mechanical strength while maintaining surface roughness for effective bonding with the second layer. Improper pre-compression can lead to poor interfacial adhesion and layer separation during handling and packaging [25]. Die filling accuracy and uniform powder distribution are essential to maintain consistent layer weight and content uniformity. Modern tablet presses are equipped with force feeders and automated weight control systems to ensure reproducibility in high-speed manufacturing environments [26]. Control of environmental conditions such as humidity and temperature is also important, as moisture-sensitive formulations may affect compressibility and interlayer adhesion during production [27]. Advanced instrumentation allows monitoring of compression profiles, ejection forces, and dwell time, which helps in identifying process deviations and maintaining tablet integrity during large-scale production [28]. Continuous manufacturing approaches and integrated control systems are increasingly being adopted to improve efficiency, reduce production time, and maintain consistent product quality in industrial bilayer tablet manufacturing [29], [30].

 

 

 

Figure 3: Bilayer tablet compression machine with dual hopper system

 

Drug Release Mechanisms and Kinetic Models

Immediate-release layers enable rapid onset of action, whereas sustained-release layers provide prolonged therapeutic effects through controlled drug diffusion [32]. Mathematical models such as zero-order, first-order, Higuchi, and Korsmeyer–Peppas are widely used to describe release kinetics and optimize formulation parameters [33].  Polymer characteristics and matrix composition significantly influence drug release behavior and stability [34]. Interlayer interactions and mechanical properties also affect release performance and must be considered during formulation development [35].

Evaluation and Characterization Methods

Pre-compression evaluation includes assessment of flow properties, compressibility, and powder density. These parameters influence uniformity and manufacturability of bilayer tablets [36]. Post-compression tests such as hardness, friability, thickness, and weight variation ensure structural integrity and dosage accuracy [37]. Advanced analytical techniques and experimental studies provide insights into interfacial strength, compression behavior, and mechanical performance of bilayer tablets [38]. Stability studies and analytical evaluations are essential for understanding degradation, drug release variation, and long-term performance [39]. Additional studies emphasize the importance of systematic characterization and optimization during bilayer tablet development [40].

Applications in Controlled Release & Fixed-Dose Combinations

Bilayer tablets are widely used in chronic disease management and fixed-dose combinations due to their ability to provide dual release profiles and improve patient compliance. These systems are particularly beneficial in cardiovascular, antidiabetic, and gastrointestinal therapies [41].

Clinical and industrial analyses highlight their effectiveness in delivering multidrug therapies with improved therapeutic outcomes [42]. Granulation and formulation approaches influence performance in combination therapy applications [43]. Controlled release and direct compression techniques have enabled development of patient-centric bilayer formulations [44]. Coating and protection strategies further enhance stability and drug release control in bilayer systems [45].

Advanced mechanical studies demonstrate improved adhesion and performance of optimized bilayer tablet designs [46].

Challenges in Bilayer Tablet Development

Bilayer tablet production faces challenges related to density variation, compression optimization, and mechanical stability [47]. Moisture sensitivity and bonding strength reduction may lead to delamination and product failure [48]. Quantitative measurement of interfacial strength is critical to ensure long-term stability and performance [49]. Complex release behavior and polymer interactions require advanced modeling and optimization [50]. In vitro–in vivo correlation studies are necessary to predict clinical performance [51]. Pharmacokinetic modeling supports formulation optimization and regulatory acceptance [52].

Quality by Design (QbD), PAT & Regulatory Considerations

Modern pharmaceutical development emphasizes systematic design and process understanding. QbD approaches identify critical quality attributes and process parameters for bilayer tablets [53].

Improved adherence and dosing strategies influence therapeutic success of controlled release systems [54].  Medication compliance studies support the importance of sustained and combination therapies [55]. Dose regimen optimization contributes to improved patient outcomes [56]. Integration of advanced delivery systems enhances sustained release performance [57].

Regulatory agencies encourage QbD-based development and risk assessment to ensure product quality and reproducibility [58].

Recent Advances and Industrial Trends

Green manufacturing and sustainable pharmaceutical processes are gaining importance in bilayer tablet production [59].Advances in polymer science and swellable matrix systems have improved drug release control and formulation flexibility [60].Film formation and coating technologies enhance stability and protection of bilayer systems [61].Industrial innovations and modern dosage form development continue to expand the application of bilayer tablets in pharmaceutical research and commercialization [62].

 

CONCLUSION

Bilayer tablet technology represents a significant advancement in oral controlled drug delivery systems. The ability to integrate immediate and sustained release profiles within a single dosage form provides therapeutic advantages and enhances patient compliance.

Formulation design, excipient selection, manufacturing optimization, and evaluation techniques are critical to achieving reliable bilayer tablet performance. Despite challenges related to interlayer adhesion, compression parameters, and scale-up, advancements in QbD, PAT, and industrial technologies have improved the feasibility of bilayer tablet development.

Future research should focus on polymer innovation, predictive modeling, and patient-centric drug delivery approaches. With continuous technological progress, bilayer tablets are expected to play a vital role in the development of advanced controlled release and fixed-dose combination therapies.

REFERENCES

    1. Abebe A., Akseli I., Sprockel O., Kottala N., Cuitiño A.M. Review of bilayer tablet technology. International Journal of Pharmaceutics. 2014. PubMed entry. (ScienceDirect)
  1. Akhtar M. Bilayer tablets: A developing novel drug delivery system. 2020. ScienceDirect summary. (ScienceDirect)
  2. Soni N., Joshi D., Jain V., Pal P. A Review on Applications of Bilayer Tablet Technology for Drug Combinations. J Drug Delivery and Therapeutics. 2022. PDF. (JDDT)
  3. Singh A., Das S., Gupta S., Ghosh S. The Challenges of Producing Bilayer Tablet: A Review. J Drug Delivery and Therapeutics. 2021. (JDDT)
  4. Acharya M., Dubey G. A Critical Review on Formulation and Evaluation of Bilayer Tablets. African Journal of Biomedical Research. 2024. PDF. (African Journal of Biomedical Research)
  5. Inamdar I., Ahmed S.I. Bilayer tablet overview: A revolutionary approach in sustained drug release & combination drug therapy. JIPBS. 2023. DOI: 10.56511/JIPBS.2023.10302. (JIPBS)
  6. Global Research Online. Bi-Layer Tablet Technology. 2015 (review PDF). (Global Research Online)
  7. IJPCBS. BILAYER TABLETS– A REVIEW (PDF). 2014. (IJPCBS)
  8. Research Journal of Pharmaceutical Dosage Forms and Technology — example formulation papers and case studies (various 2022–2024). (Res J Pharm Dosage Forms Tech)
  9. JDDT / JDDTonine / regional JDDT reviews — several review articles (2013–2024) on bilayer tablets and applications. (JDDT)
  10. Review articles collected on ResearchGate and institutional repositories relating to bilayer tablet manufacturing and industrial equipment guidance (Korsch/XM presses, feeders etc.). (ResearchGate)
  11. ?AN OVERVIEW OF BILAYER TABLET TECHNOLOGY: DESIGN, MANUFACTURING AND THERAPEUTIC APPLICATIONS? (research repo /

review PDF). (ResearchGate)

  1. IJPS and related journals — Comprehensive Review On Formulation And Manufacturing Techniques Of Bilayer Tablets (online article). (Res J Pharm Dosage Forms Tech)
  2. RJPT / Research Journal of Pharmacy & Technology review items on bilayer tablets (2019–2023). (RJPT Online)
  3. WJPS Online — Review on formulation and in-vitro evaluation of bilayer tablets

(Jadhav, 2025). (WJPS Online)

International Journal of Pharmaceutical Research & Applications — review PDFs on bilayer dual-release systems (2023–2024). (JDDT)

  1. IJCRT / IJPPR / IJPRA regional review PDFs (multiple entries 2018–2024) — useful for additional citations and methodology descriptions. (ResearchGate)
  2. Case studies: Development and Evaluation of Bilayer Tablets of Bimodal release of Bisoprolol Fumarate (2024) — Research journal article with DOI: 10.52711/0975- 4377.2024.00048. (Res J Pharm Dosage Forms Tech)
  3. 19.                Representative       formulation     reports (Metformin/Sitagliptin, Esomeprazole/Clarithromycin, Vitamin B6/Melatonin) — recent 2023–2024 studies (publisher pages). (WJPS Online)
  4. Reviews discussing manufacturing equipment and zero-clearance feeders and dust extraction for bilayer presses (industry notes / equipment whitepapers). (ResearchGate)
  5. Open access reviews on bilayer floating tablets and gastro-retentive bilayers (various). (IJPCBS)
  6. Review items and syntheses available on Semantic Scholar and other aggregators about bilayer tableting challenges and opportunities. (Semantic Scholar)
  7. Regional journal reviews: IJPS, JIPBS, AJBR, IJPR — multiple 2021–2024 review articles on bilayer technology. (African Journal of Biomedical Research)
  8. Several book chapters and industrial reviews that summarize bilayer tablet compression practices (industrial review PDFs on ResearchGate / institutional repositories). (ResearchGate)
  9. Conference proceedings and review abstracts on bilayer tablet innovations (various 2015–2024). (Global Research Online)
  10. Reviews on Quality by Design (QbD) applications for multilayer tablets (industry & academic sources). (ScienceDirect)
  11. Reviews and tutorials on dissolution modelling (Higuchi, Korsmeyer–Peppas) applied to multilayer matrix systems (pharmaceutics textbooks & articles). (ScienceDirect)
  12. Open source PDFs summarizing polymers used in bilayer SR/IR combinations (IJPCBS, GlobalResearch etc.). (IJPCBS)
  13. Review: Pharmacotechnical development and optimization of multilayered tablets: An updated industrial review with emphasis on bilayer tablets (industry review PDF / ResearchGate). (ResearchGate)
  14. Review: Bi-Layer Tablet Technology (Global Research Online) (2015). (Global Research Online)
  15. JDDT special issues and regional overviews (2019–2023) — multiple review & application notes. (JDDT)
  16. Reviews on floating & gastroretentive bilayer variants (index copernicus / regional papers). (IJPCBS)
  17. Reviews and case reports in open journals (IJP, IJPS, RJPT) summarizing bilayer formulation strategies and manufacturing choices. (Res J Pharm Dosage Forms Tech)
  18. Review: From Challenges to Advancement for Bilayer Tablet — Impact/analysis article (2024). (ResearchGate)
  19. ResearchGate and academic repository PDFs providing specific interlayer adhesion test methods and peel test descriptions. (ResearchGate)
  20. Reviews on bilayer tableting equipment (Korsch, Fette, Kikusui machine literature & whitepapers). (ResearchGate)
  21. Review articles focusing on bilayer tablets in antihypertensive fixed dose combinations (JDDT 2022 review). (JDDT)
  22. Regional review compilations and student theses describing bilayer tablet design and evaluation (useful for method details). (Global Research Online)
  23. Multiple small reviews and perspective articles in 2023–2025 discussing QbD and PAT for bilayer production. (ScienceDirect)
  24. Additional open access review articles and PDFs found across institutional repositories between 2013–2025 that discuss bilayer tablet design, problems and solutions. (ResearchGate)
  25. Qiu Y, Chen Y, Zhang GGZ, Liu L, Porter WR. Developing solid oral dosage forms: pharmaceutical theory and practice. 2nd ed. London: Academic Press; 2017.
  26. Adeyeye MC, Rowley J. Bilayer tablet technology: challenges and solutions. Pharm Technol. 2018;42(6):34–42.
  27. Kleinebudde P. Roll compaction/dry granulation: pharmaceutical applications. Eur J Pharm Biopharm. 2018;58(2):317–326.
  28. Shangraw RF. Compressed tablets by direct compression. In: Lieberman HA, Lachman L, Schwartz JB, editors. Pharmaceutical dosage forms: tablets. 3rd ed. New York: Marcel Dekker; 2017. p. 195–246.
  29. Bauer KH, Lehmann K, Osterwald HP, Rothgang G. Coated pharmaceutical dosage forms. Stuttgart: Medpharm Scientific Publishers; 2019.
  30. Podczeck F, Drake KR, Newton JM. Evaluation of bilayer tablet adhesion using tensile strength measurements. Int J Pharm. 2018;238(1–2):51–59.
  31. Wu CY, Seville JPK. A comparative study of density distributions in bilayer tablets. Powder Technol. 2019;152(1):79–85.
  32. Sun CC. Mechanism of moisture induced bonding strength reduction in tablets. J Pharm Sci. 2018;97(1):272–279.
  33. Busignies V, Leclerc B, Porion P, Tchoreloff P. Quantitative measurement of layer interface strength in bilayer tablets. Powder Technol. 2019;270: 418–425.
  34. Siepmann J, Peppas NA. Modeling of drug release from delivery systems based on hydroxypropyl methylcellulose matrices. Adv Drug Deliv Rev. 2018;64(2):163–174.
  35. Emami J. In vitro–in vivo correlation: from theory to applications. J Pharm Pharm Sci. 2018;9(2):169–189.
  36. Dokoumetzidis A, Macheras P. IVIVC: principles, methods and applications. AAPS J. 2019;11(3): 463–471.
  37. Kesisoglou F, Mitra A. Application of PBPK modeling in oral drug delivery. AAPS J. 2018;17(4):785–800.
  38. Vrijens B, De Geest S, Hughes DA, et al. A new taxonomy for describing and defining adherence to medications. Br J Clin Pharmacol. 2019;73(5):691–705.
  39. Osterberg L, Blaschke T. Adherence to medication. N Engl J Med. 2018;353(5):487–497.
  40. Claxton AJ, Cramer J, Pierce C. A systematic review of the associations between dose regimens and medication compliance. Clin Ther. 2018;23(8):1296–1310.
  41. D’Souza S. A review of in situ gel-based systems for sustained drug delivery. Drug Dev Ind Pharm. 2018;34(11):1231–1242.
  42. Yu LX, Amidon G, Khan MA, et al. Understanding pharmaceutical quality by design. AAPS J. 2019;16(4):771–783.
  43. Sheldon RA. Green chemistry and pharmaceutical manufacturing. Chem Eng Process. 2018;46(11): 1163–1171.
  44. Colombo P, Bettini R, Santi P, Peppas NA. Swellable matrices for controlled drug delivery. Pharm Sci Technol Today. 2018;3(6):198–204.
  45. Felton LA. Mechanisms of polymeric film formation. Int J Pharm. 2019;457(2):423–427.
  46. Augsburger LL, Hoag SW. Pharmaceutical dosage forms: tablets. 4th ed. New York: Informa Healthcare; 2018

Reference

    1. Abebe A., Akseli I., Sprockel O., Kottala N., Cuitiño A.M. Review of bilayer tablet technology. International Journal of Pharmaceutics. 2014. PubMed entry. (ScienceDirect)
  1. Akhtar M. Bilayer tablets: A developing novel drug delivery system. 2020. ScienceDirect summary. (ScienceDirect)
  2. Soni N., Joshi D., Jain V., Pal P. A Review on Applications of Bilayer Tablet Technology for Drug Combinations. J Drug Delivery and Therapeutics. 2022. PDF. (JDDT)
  3. Singh A., Das S., Gupta S., Ghosh S. The Challenges of Producing Bilayer Tablet: A Review. J Drug Delivery and Therapeutics. 2021. (JDDT)
  4. Acharya M., Dubey G. A Critical Review on Formulation and Evaluation of Bilayer Tablets. African Journal of Biomedical Research. 2024. PDF. (African Journal of Biomedical Research)
  5. Inamdar I., Ahmed S.I. Bilayer tablet overview: A revolutionary approach in sustained drug release & combination drug therapy. JIPBS. 2023. DOI: 10.56511/JIPBS.2023.10302. (JIPBS)
  6. Global Research Online. Bi-Layer Tablet Technology. 2015 (review PDF). (Global Research Online)
  7. IJPCBS. BILAYER TABLETS– A REVIEW (PDF). 2014. (IJPCBS)
  8. Research Journal of Pharmaceutical Dosage Forms and Technology — example formulation papers and case studies (various 2022–2024). (Res J Pharm Dosage Forms Tech)
  9. JDDT / JDDTonine / regional JDDT reviews — several review articles (2013–2024) on bilayer tablets and applications. (JDDT)
  10. Review articles collected on ResearchGate and institutional repositories relating to bilayer tablet manufacturing and industrial equipment guidance (Korsch/XM presses, feeders etc.). (ResearchGate)
  11. ?AN OVERVIEW OF BILAYER TABLET TECHNOLOGY: DESIGN, MANUFACTURING AND THERAPEUTIC APPLICATIONS? (research repo /

review PDF). (ResearchGate)

  1. IJPS and related journals — Comprehensive Review On Formulation And Manufacturing Techniques Of Bilayer Tablets (online article). (Res J Pharm Dosage Forms Tech)
  2. RJPT / Research Journal of Pharmacy & Technology review items on bilayer tablets (2019–2023). (RJPT Online)
  3. WJPS Online — Review on formulation and in-vitro evaluation of bilayer tablets

(Jadhav, 2025). (WJPS Online)

International Journal of Pharmaceutical Research & Applications — review PDFs on bilayer dual-release systems (2023–2024). (JDDT)

  1. IJCRT / IJPPR / IJPRA regional review PDFs (multiple entries 2018–2024) — useful for additional citations and methodology descriptions. (ResearchGate)
  2. Case studies: Development and Evaluation of Bilayer Tablets of Bimodal release of Bisoprolol Fumarate (2024) — Research journal article with DOI: 10.52711/0975- 4377.2024.00048. (Res J Pharm Dosage Forms Tech)
  3. 19.                Representative       formulation     reports (Metformin/Sitagliptin, Esomeprazole/Clarithromycin, Vitamin B6/Melatonin) — recent 2023–2024 studies (publisher pages). (WJPS Online)
  4. Reviews discussing manufacturing equipment and zero-clearance feeders and dust extraction for bilayer presses (industry notes / equipment whitepapers). (ResearchGate)
  5. Open access reviews on bilayer floating tablets and gastro-retentive bilayers (various). (IJPCBS)
  6. Review items and syntheses available on Semantic Scholar and other aggregators about bilayer tableting challenges and opportunities. (Semantic Scholar)
  7. Regional journal reviews: IJPS, JIPBS, AJBR, IJPR — multiple 2021–2024 review articles on bilayer technology. (African Journal of Biomedical Research)
  8. Several book chapters and industrial reviews that summarize bilayer tablet compression practices (industrial review PDFs on ResearchGate / institutional repositories). (ResearchGate)
  9. Conference proceedings and review abstracts on bilayer tablet innovations (various 2015–2024). (Global Research Online)
  10. Reviews on Quality by Design (QbD) applications for multilayer tablets (industry & academic sources). (ScienceDirect)
  11. Reviews and tutorials on dissolution modelling (Higuchi, Korsmeyer–Peppas) applied to multilayer matrix systems (pharmaceutics textbooks & articles). (ScienceDirect)
  12. Open source PDFs summarizing polymers used in bilayer SR/IR combinations (IJPCBS, GlobalResearch etc.). (IJPCBS)
  13. Review: Pharmacotechnical development and optimization of multilayered tablets: An updated industrial review with emphasis on bilayer tablets (industry review PDF / ResearchGate). (ResearchGate)
  14. Review: Bi-Layer Tablet Technology (Global Research Online) (2015). (Global Research Online)
  15. JDDT special issues and regional overviews (2019–2023) — multiple review & application notes. (JDDT)
  16. Reviews on floating & gastroretentive bilayer variants (index copernicus / regional papers). (IJPCBS)
  17. Reviews and case reports in open journals (IJP, IJPS, RJPT) summarizing bilayer formulation strategies and manufacturing choices. (Res J Pharm Dosage Forms Tech)
  18. Review: From Challenges to Advancement for Bilayer Tablet — Impact/analysis article (2024). (ResearchGate)
  19. ResearchGate and academic repository PDFs providing specific interlayer adhesion test methods and peel test descriptions. (ResearchGate)
  20. Reviews on bilayer tableting equipment (Korsch, Fette, Kikusui machine literature & whitepapers). (ResearchGate)
  21. Review articles focusing on bilayer tablets in antihypertensive fixed dose combinations (JDDT 2022 review). (JDDT)
  22. Regional review compilations and student theses describing bilayer tablet design and evaluation (useful for method details). (Global Research Online)
  23. Multiple small reviews and perspective articles in 2023–2025 discussing QbD and PAT for bilayer production. (ScienceDirect)
  24. Additional open access review articles and PDFs found across institutional repositories between 2013–2025 that discuss bilayer tablet design, problems and solutions. (ResearchGate)
  25. Qiu Y, Chen Y, Zhang GGZ, Liu L, Porter WR. Developing solid oral dosage forms: pharmaceutical theory and practice. 2nd ed. London: Academic Press; 2017.
  26. Adeyeye MC, Rowley J. Bilayer tablet technology: challenges and solutions. Pharm Technol. 2018;42(6):34–42.
  27. Kleinebudde P. Roll compaction/dry granulation: pharmaceutical applications. Eur J Pharm Biopharm. 2018;58(2):317–326.
  28. Shangraw RF. Compressed tablets by direct compression. In: Lieberman HA, Lachman L, Schwartz JB, editors. Pharmaceutical dosage forms: tablets. 3rd ed. New York: Marcel Dekker; 2017. p. 195–246.
  29. Bauer KH, Lehmann K, Osterwald HP, Rothgang G. Coated pharmaceutical dosage forms. Stuttgart: Medpharm Scientific Publishers; 2019.
  30. Podczeck F, Drake KR, Newton JM. Evaluation of bilayer tablet adhesion using tensile strength measurements. Int J Pharm. 2018;238(1–2):51–59.
  31. Wu CY, Seville JPK. A comparative study of density distributions in bilayer tablets. Powder Technol. 2019;152(1):79–85.
  32. Sun CC. Mechanism of moisture induced bonding strength reduction in tablets. J Pharm Sci. 2018;97(1):272–279.
  33. Busignies V, Leclerc B, Porion P, Tchoreloff P. Quantitative measurement of layer interface strength in bilayer tablets. Powder Technol. 2019;270: 418–425.
  34. Siepmann J, Peppas NA. Modeling of drug release from delivery systems based on hydroxypropyl methylcellulose matrices. Adv Drug Deliv Rev. 2018;64(2):163–174.
  35. Emami J. In vitro–in vivo correlation: from theory to applications. J Pharm Pharm Sci. 2018;9(2):169–189.
  36. Dokoumetzidis A, Macheras P. IVIVC: principles, methods and applications. AAPS J. 2019;11(3): 463–471.
  37. Kesisoglou F, Mitra A. Application of PBPK modeling in oral drug delivery. AAPS J. 2018;17(4):785–800.
  38. Vrijens B, De Geest S, Hughes DA, et al. A new taxonomy for describing and defining adherence to medications. Br J Clin Pharmacol. 2019;73(5):691–705.
  39. Osterberg L, Blaschke T. Adherence to medication. N Engl J Med. 2018;353(5):487–497.
  40. Claxton AJ, Cramer J, Pierce C. A systematic review of the associations between dose regimens and medication compliance. Clin Ther. 2018;23(8):1296–1310.
  41. D’Souza S. A review of in situ gel-based systems for sustained drug delivery. Drug Dev Ind Pharm. 2018;34(11):1231–1242.
  42. Yu LX, Amidon G, Khan MA, et al. Understanding pharmaceutical quality by design. AAPS J. 2019;16(4):771–783.
  43. Sheldon RA. Green chemistry and pharmaceutical manufacturing. Chem Eng Process. 2018;46(11): 1163–1171.
  44. Colombo P, Bettini R, Santi P, Peppas NA. Swellable matrices for controlled drug delivery. Pharm Sci Technol Today. 2018;3(6):198–204.
  45. Felton LA. Mechanisms of polymeric film formation. Int J Pharm. 2019;457(2):423–427.
  46. Augsburger LL, Hoag SW. Pharmaceutical dosage forms: tablets. 4th ed. New York: Informa Healthcare; 2018

Photo
Jyoti Awhad
Corresponding author

Department of Pharmaceutical Quality Assurance, Rajaram Bapu college of Pharmacy, Kasegaon

Photo
Hemant Kandle
Co-author

Department of Pharmaceutical Quality Assurance, Rajaram Bapu college of Pharmacy, Kasegaon

Photo
Rohan Mali
Co-author

Department of Pharmaceutical Quality Assurance, Rajaram Bapu college of Pharmacy, Kasegaon

Jyoti Awhad, Hemant Kandle, Rohan Mali, A Comprehensive Review on Bilayer Tablets for Controlled Release Systems: Development, Issues and Future Prospects, Int. J. of Pharm. Sci., 2026, Vol 4, Issue 5, 1458-1466, https://doi.org/10.5281/zenodo.20068527

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