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Abstract

Mosquito-borne diseases, particularly malaria, continue to pose a major global public health challenge, especially in tropical and subtropical regions. The present study focuses on the formulation and evaluation of a herbal mosquito repellent cream using natural phytochemicals as a safe and eco-friendly alternative to synthetic mosquito repellents. The oil-in-water (O/W) emulsion cream was prepared using a combination of natural ingredients including citronella oil, eucalyptus oil, clove oil, neem oil, and Phyllanthus emblica extract. The oil phase and aqueous phase were heated separately, followed by gradual emulsification with continuous stirring and cooling to obtain a stable cream formulation.Future research may focus on microencapsulation of essential oils to extend the duration of protection, large-scale clinical trials in malaria-endemic regions, and the development of specialized formulations for children and individuals with sensitive skin

Keywords

Citronella oil, Neem oil, Eucalyptus oil, Clove oil, Oil-in-water emulsion, Malaria prevention, Skin-friendly formulation

Introduction

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Herbal mosquito repellents prepared from plant-derived essential oils have gained considerable attention due to their biodegradability, low toxicity, pleasant fragrance, and minimal side effects. Essential oils such as citronella oil, eucalyptus oil, clove oil, and neem oil possess natural mosquito-repellent properties by masking human odour and interfering with the mosquito’s ability to detect its host. In addition, Phyllanthus emblica (Alma) extract provides antioxidant and skin-protective benefits, making the formulation more suitable for topical application.

In the present study, an oil-in-water (O/W) herbal mosquito repellent cream was formulated using selected natural phytochemicals and evaluated for its physicochemical properties, skin compatibility, stability, and mosquito repellency. The prepared cream showed good spreadability, a skin-friendly pH, no phase separation or skin irritation, and provided effective mosquito protection for approximately 2–3 hours. This formulation demonstrates the potential of herbal ingredients as a safe, effective, and environmentally friendly alternative to conventional mosquito repellent cream .

Composition of cream

Ingredients

%w/w composition

Citronella oil

3.0

Eucalyptus oil

2.0

Neem oil

2.0

Clove oil

1.0

Phyllanthus emblica extract

1.0

Pharmacognostic Profile of Ingredients Used in the Formulation

 

Ingredients

Biological sources

Chemical constituents

Medicinal uses

 


Citronella oil

 

Volatile oil obtained from the leaves of Cymbopogon nardus or Cymbopogon winterianus (Family: Poaceae)

Citronellal, Citronellol, Geraniol, Limonene

Natural mosquito repellent, insect repellent, antimicrobial, provides pleasant fragrance.

 


Eucalyptus oil

 

Volatile oil obtained from fresh leaves of Eucalyptus globules (Family: Myrtaceae)

1,8-Cineole (Eucalyptol), α-Pinene, Limonene, Terpineol

1,8-Cineole (Eucalyptol), α-Pinene, Limonene, Terpineol

Mosquito repellent, antiseptic, anti-inflammatory, cooling effect, antimicrobial.

 


Clove oil

 

Volatile oil obtained from dried flower buds of Syzygium aromaticum (Family: Myrtaceae)

Eugenol, Eugenyl acetate, β-Caryophyllene

Mosquito repellent, analgesic, antimicrobial, antioxidant, preservative.

Eugenol, Eugenyl acetate, β-Caryophyllene

Mosquito repellent, analgesic, antimicrobial, antioxidant, preservative.

 


Neem oil

 

Fixed oil obtained from the seeds of Azadirachta indica (Family: Meliaceae)

Azadirachtin, Nimbin, Nimbidin, Salannin

Natural insect repellent, insecticidal, antifungal, antibacterial, anti-inflammatory, skin protective.

 


Phyllanthus emblica extract (Amla)

 

 

Dried fruits of Phyllanthus emblica Linn. (Family: Phyllanthaceae)

Vitamin C (Ascorbic acid), Gallic acid, Ellagic acid, Emblicanin A & B, Tannins

Antioxidant, skin nourishing, anti-inflammatory, antimicrobial, promotes skin health and protects against oxidative damage.

 

Formula : For making 20 gm of cream

Ingredients

Quantity

Citronella oil

0.60ml

Eucalyptus oil

0.40ml

Clove oil

0.20 ml

Neem oil

0.40ml

Phyllanthus emblica (amla) extract

0.20ml

Emulsifying wax

2 gm

Cetyl alcohol

1 gm

Glycerine

2 ml

Purified water

13.20ml

 

Procedure:

Step 1: Weighing of Ingredients

Accurately weigh all ingredients according to the formulation for 20 g cream.

Step 2: Preparation of Oil Phase

Transfer emulsifying wax and cetyl alcohol into a clean beaker. Add citronella oil, eucalyptus oil, clove oil, and neem oil. Heat the mixture on a water bath at 70–75°C until the wax melts completely and a clear oil phase is obtained.

Step 3: Preparation of Aqueous Phase

In another beaker, dissolve glycerin in the required quantity of purified water. Add the Phyllanthus emblica extract and stir until uniformly dispersed. Heat the aqueous phase separately to 70–75°C.

Step 4: Emulsification

Slowly add the hot aqueous phase to the hot oil phase with continuous stirring using a magnetic stirrer or glass rod. Stir continuously for 10–15 minutes until a smooth and homogeneous oil-in-water (O/W) emulsion is formed.

Step 5: Cooling

Continue stirring while allowing the emulsion to cool gradually to room temperature (25–30°C). Continuous stirring during cooling prevents phase separation and produces a smooth cream.

Step 6: Homogenization

Homogenize the cream for 3–5 minutes to improve uniformity, texture, viscosity, and spread ability.

Step 7: Filling and Storage

Transfer the prepared cream into a clean, dry, airtight cream container. Label the container with required ingredients.

Storage condition

Store the cream in a cool, dry place away from direct sunlight.

 

 

 

 

Evaluation parameters:

 

Parameters

Method

Observation

Appearance

Visual inspection

Smooth, homogeneous, off-white cream with no lumps.

color

Visual inspection

Off-white to pale cream.

odour

Organoleptic evaluation

Pleasant herbal aroma due to essential oils.

PH

Measured using a digital pH meter (1 g cream dispersed in 10 mL distilled water)

4.7(eco friendly)

Viscosity

Measured using a Brookfield Viscometer

Smooth, optimum viscosity suitable for topical application.

Spreadability

Slide method

Cream spreads easily with uniform consistency.

Homogeneity

Visual examination after application on a glass slide

Uniform texture, free from coarse particles and lumps.

Uniform texture, free from coarse particles and lumps.

Washability

Wash with tap water

Easily washable without leaving excessive residue.

Phase Separation

Stored at room temperature for 30 days

No phase separation observed.

Skin Irritation Test (Patch Test)

Applied on a small area of skin for 24 hours

No redness, itching, swelling, or irritation observed.

Mosquito Repellency Test

Arm-in-cage or cage test

Effective mosquito repellency for 2–3 hours.

Stability Study

Stored at room temperature and accelerated conditions

No significant change In colour, odour, pH, viscosity, or phase separation.

Extrudability (if packed in tube)

Measure ease of cream extrusion

Cream extrudes uniformly with slight pressure.

 

CONCLUSION

The present study successfully formulated and evaluated a herbal mosquito repellent cream using natural phytochemicals, including citronella oil, eucalyptus oil, clove oil, neem oil, and Phyllanthus emblica extract. The cream was prepared using the oil-in-water (O/W) emulsion technique and exhibited desirable physicochemical properties such as smooth texture, good spreadability, pleasant odour, skin-friendly pH (4.7), and no phase separation. The formulation was found to be non-irritant during the skin patch test and remained stable throughout the evaluation period. Further studies involving long-term stability testing, optimization of the formulation, and large-scale clinical evaluation are recommended to enhance its efficacy and commercial applicability.

RESULT

The herbal mosquito repellent cream was successfully formulated using an oil-in-water (O/W) emulsion method. The prepared cream was smooth, homogeneous, and off-white in appearance with a pleasant herbal odour. It exhibited a skin-friendly pH of 4.7 and showed good spreadability without phase separation. The formulation remained stable throughout the evaluation period and caused no skin irritation during the patch test. Mosquito repellency studies indicated effective protection for approximately 2–3 hours. The cream demonstrated satisfactory physicochemical properties, good stability, and effective mosquito repellent activity, suggesting its suitability for topical application.

REFERENCES

  1. Govindarajan M, Rajeswary M. Mosquito repellent activity of essential oils: A review. Parasitol Res. 2018;117(12):3887–3906.
  2. Maia MF, Moore SJ. Plant-based insect repellents: A review of their efficacy, development and testing. Malar J. 2011;10(Suppl 1):S11.
  3. Amer A, Mehlhorn H. Repellency effect of forty-one essential oils against Aedes, Anopheles, and Culex mosquitoes. Parasitol Res. 2006;99(4):478–490.
  4. World Health Organization (WHO). World Malaria Report 2023. Geneva: World Health Organization.
  5. Kokate CK, Purohit AP, Gokhale SB. Pharmacognosy. 57th ed. Pune: Nirali Prakashan.Indian Pharmacopoeia Commission. Indian Pharmacopoeia 2022. Ghaziabad: IPC.

Reference

  1. Govindarajan M, Rajeswary M. Mosquito repellent activity of essential oils: A review. Parasitol Res. 2018;117(12):3887–3906.
  2. Maia MF, Moore SJ. Plant-based insect repellents: A review of their efficacy, development and testing. Malar J. 2011;10(Suppl 1):S11.
  3. Amer A, Mehlhorn H. Repellency effect of forty-one essential oils against Aedes, Anopheles, and Culex mosquitoes. Parasitol Res. 2006;99(4):478–490.
  4. World Health Organization (WHO). World Malaria Report 2023. Geneva: World Health Organization.
  5. Kokate CK, Purohit AP, Gokhale SB. Pharmacognosy. 57th ed. Pune: Nirali Prakashan.Indian Pharmacopoeia Commission. Indian Pharmacopoeia 2022. Ghaziabad: IPC.

Photo
P K Lavare
Corresponding author

Pravara Rural College Of Pharmacy, Pravaranagre,Loni, India.

Photo
P C Kunde
Co-author

Pravara Rural College Of Pharmacy, Pravaranagre,Loni, India.

P K Lavare, P C Kunde, Herbal Mosquito Repellent Cream, Int. J. of Pharm. Sci., 2026, Vol 4, Issue 8, 764-768, https://doi.org/10.5281/zenodo.21802765

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